From Chemistry Towards Technology Step-By-Step From Chemistry Towards Technology Step-By-Step От химии к технологии шаг за шагом 2782-1900 109568 10.52957/2782-1900-2025-6-4-72-82 Научные статьи Scientific articles Научные статьи Dopamine-driven coloration technologies: a knowledge structuring built on Citavi and artificial intelligence Dopamine-driven coloration technologies: a knowledge structuring built on Citavi and artificial intelligence Телегин Феликс Юрьевич Telegin Felix Yurievich f.telegin@mail.ru

доктор химических наук;

doctor of chemical sciences;

 Никифорова Татьяна Евгеньевна Nokoforova Tatyana Evgenjevna tatianaenik@mail.ru

доктор химических наук;

doctor of chemical sciences;

 Ran Jianhua Ran Jianhua jhran@wtu.edu.cn Пряжникова Виктория Георгиевна Pryazhnikova Victoria Georgievna prajnikova@mail.ru Ивановский государственный химико-технологический университет Ivanovo State University of Chemistry and Technology Wuhan Textile University Wuhan Китайская Народная Республика Wuhan Textile University Wuhan China 22 12 2025 22 12 2025 6 4 72 82 10 09 2025 19 12 2025 https://chemintech.ru/en/nauka/article/109568/view

The interdisciplinary field of dopamine-mediated coloration, spanning materials science, biomimetics, and sustainable chemistry, has experienced rapid growth, making comprehensive literature synthesis increasingly challenging. This paper presents a novel methodology for transforming the reference management software Citavi into a structured knowledge system, enabling both manual and AI-augmented trend analysis. We curated and annotated over 1,000 publications, with particular focus on dopamine and polydopamine in textile functionalization and coloration. Structuring via custom taxonomies (e.g., substrate type, deposition method, durability metrics) enabled AI-driven synthesis using Qwen3-Max. Key insights include: (1) PDA’s role as a universal textile modifier enhancing dye fastness, enabling structural color, and imparting antimicrobial/UV functions; (2) enzymatic (laccase-mediated) DA polymerization as an emerging green alternative; (3) under-explored potential in wool and scalability studies. AI insights were reintegrated into Citavi as “AI Insight Notes,” creating a dynamic human-AI collaborative environment. This approach offers a reproducible framework for domain mapping in fast-evolving fields.

The interdisciplinary field of dopamine-mediated coloration, spanning materials science, biomimetics, and sustainable chemistry, has experienced rapid growth, making comprehensive literature synthesis increasingly challenging. This paper presents a novel methodology for transforming the reference management software Citavi into a structured knowledge system, enabling both manual and AI-augmented trend analysis. We curated and annotated over 1,000 publications, with particular focus on dopamine and polydopamine in textile functionalization and coloration. Structuring via custom taxonomies (e.g., substrate type, deposition method, durability metrics) enabled AI-driven synthesis using Qwen3-Max. Key insights include: (1) PDA’s role as a universal textile modifier enhancing dye fastness, enabling structural color, and imparting antimicrobial/UV functions; (2) enzymatic (laccase-mediated) DA polymerization as an emerging green alternative; (3) under-explored potential in wool and scalability studies. AI insights were reintegrated into Citavi as “AI Insight Notes,” creating a dynamic human-AI collaborative environment. This approach offers a reproducible framework for domain mapping in fast-evolving fields.

 dopamine polydopamine coloration Citavi knowledge system trend analysis AI in research Qwen3-Max materials science bibliometric synthesis dopamine polydopamine coloration Citavi knowledge system trend analysis AI in research Qwen3-Max materials science bibliometric synthesis This work was funded by the Ministry of Science and Higher Education of the Russian Federation (Project No. FZZW–2024–0004).

Lee H., Dellatore S. M., Miller W. M., Messersmith P. B. A review on heavy metal pollution, toxicity and remedial measures: current trends and future perspectives. Science, 2007, 318, 26–430. DOI: 10.1126/science.1147241. Lee H., Dellatore S. M., Miller W. M., Messersmith P. B. A review on heavy metal pollution, toxicity and remedial measures: current trends and future perspectives. Science, 2007, 318, 26–430. DOI: 10.1126/science.1147241. Wei X., Wang Y., Chen J., Liu Z., Xu F., He X., Li H., Zhou Y. Fabrication of di-selective adsorption platform based on deep eutectic solvent stabilized magnetic polydopamine: Achieving di-selectivity conversion through adding CaCl₂. Chem. Eng. J., 2021, 421, 127815. DOI: 10.1016/j.cej.2020.127815. Wei X., Wang Y., Chen J., Liu Z., Xu F., He X., Li H., Zhou Y. Fabrication of di-selective adsorption platform based on deep eutectic solvent stabilized magnetic polydopamine: Achieving di-selectivity conversion through adding CaCl₂. Chem. Eng. J., 2021, 421, 127815. DOI: 10.1016/j.cej.2020.127815. Mahmoodi N. M., Najafi F. Preparation of surface modified zinc oxide nanoparticle with high capacity dye removal ability. Mater. Res. Bull., 2012, 47, 1–8. DOI: 10.1016/j.materresbull.2012.03.026. Mahmoodi N. M., Najafi F. Preparation of surface modified zinc oxide nanoparticle with high capacity dye removal ability. Mater. Res. Bull., 2012, 47, 1–8. DOI: 10.1016/j.materresbull.2012.03.026. Vokurova D. A., Nikiforova T. Ye. Modelirovaniye protsessa adsorbtsii ionov Cu(II) na tsellyulozosoderzhashchikh sorbentakh. XLVII Mezhdunarodnaya nauchno-prakticheskaya konferentsiya. Petrozavodsk, 2025, P.79–83. Vokurova D. A., Nikiforova T. Ye. Modelirovaniye protsessa adsorbtsii ionov Cu(II) na tsellyulozosoderzhashchikh sorbentakh. XLVII Mezhdunarodnaya nauchno-prakticheskaya konferentsiya. Petrozavodsk, 2025, P.79–83. Jiang W., Yang X., Deng J., Zhang L., Liu Y. Polydopamine-based materials applied in Li-ion batteries: a review. J. Mater. Sci., 2021, 56, 19359–19382. DOI: 10.1007/s10853-021-06536-3. Jiang W., Yang X., Deng J., Zhang L., Liu Y. Polydopamine-based materials applied in Li-ion batteries: a review. J. Mater. Sci., 2021, 56, 19359–19382. DOI: 10.1007/s10853-021-06536-3. Ahmad N., Zhang X., Yang S., Zhang D., Wang J., Zafar S. u., Li Y., Zhang Y., Hussain S., Cheng Z., Kumaresan A., Zhou H. Polydopamine/ZnO electron transport layers enhance charge extraction in inverted non-fullerene organic solar cells. J. Mater. Chem. C, 2019, 7, 10795–10801. DOI: 10.1039/C9TC02781E. Ahmad N., Zhang X., Yang S., Zhang D., Wang J., Zafar S. u., Li Y., Zhang Y., Hussain S., Cheng Z., Kumaresan A., Zhou H. Polydopamine/ZnO electron transport layers enhance charge extraction in inverted non-fullerene organic solar cells. J. Mater. Chem. C, 2019, 7, 10795–10801. DOI: 10.1039/C9TC02781E. Aguilar-Ferrer D., Szewczyk J., Coy E. Recent developments in polydopamine-based photocatalytic nanocomposites for energy production: Physico-chemical properties and perspectives. Catal. Today, 2022, 397–399, 316–349. DOI: 10.1016/j.cattod.2021.08.016. Aguilar-Ferrer D., Szewczyk J., Coy E. Recent developments in polydopamine-based photocatalytic nanocomposites for energy production: Physico-chemical properties and perspectives. Catal. Today, 2022, 397–399, 316–349. DOI: 10.1016/j.cattod.2021.08.016. Cheng X. Q., Wang Z. X., Guo J., Ma J., Shao L. Designing Multifunctional Coatings for Cost-Effectively Sustainable Water Remediation. ACS Sustainable Chem. Eng., 2018, 6, 1881–1890. DOI: 10.1021/acssuschemeng.7b03296. Cheng X. Q., Wang Z. X., Guo J., Ma J., Shao L. Designing Multifunctional Coatings for Cost-Effectively Sustainable Water Remediation. ACS Sustainable Chem. Eng., 2018, 6, 1881–1890. DOI: 10.1021/acssuschemeng.7b03296. Ran J., Bi S., Jiang H., Zhang Y., Li R. Core–shell BiVO₄@PDA composite photocatalysts on cotton fabrics for highly efficient photodegradation under visible light. Cellulose, 2019, 26, 6259–6273. DOI: 10.1007/s10570-019-02535-5. Ran J., Bi S., Jiang H., Zhang Y., Li R. Core–shell BiVO₄@PDA composite photocatalysts on cotton fabrics for highly efficient photodegradation under visible light. Cellulose, 2019, 26, 6259–6273. DOI: 10.1007/s10570-019-02535-5. Liu Y., Ai K., Lu L. Polydopamine and Its Derivative Materials: Synthesis and Promising Applications in Energy, Environmental, and Biomedical Fields. Chem. Rev., 2014, 114, 5057–5115. DOI: 10.1021/cr400407a. Liu Y., Ai K., Lu L. Polydopamine and Its Derivative Materials: Synthesis and Promising Applications in Energy, Environmental, and Biomedical Fields. Chem. Rev., 2014, 114, 5057–5115. DOI: 10.1021/cr400407a. Barclay T. G., Hegab H. M., Clarke S. R., Ginic-Markovic M. Versatile Surface Modification Using Polydopamine and Related Polycatecholamines: Chemistry, Structure, and Applications. Adv. Mater. Interfaces, 2017, 4, 1601192. DOI: 10.1002/admi.201601192. Barclay T. G., Hegab H. M., Clarke S. R., Ginic-Markovic M. Versatile Surface Modification Using Polydopamine and Related Polycatecholamines: Chemistry, Structure, and Applications. Adv. Mater. Interfaces, 2017, 4, 1601192. DOI: 10.1002/admi.201601192. Kohri M., Nannichi Y., Taniguchi T., Miyazaki T., Kojima Y., Fujii S., Ishihara M., Matsuoka H., Kunitake T. Biomimetic non-iridescent structural color materials from polydopamine black particles that mimic melanin granules. J. Mater. Chem. C, 2015, 3, 720–724. DOI: 10.1039/C4TC02383H. Kohri M., Nannichi Y., Taniguchi T., Miyazaki T., Kojima Y., Fujii S., Ishihara M., Matsuoka H., Kunitake T. Biomimetic non-iridescent structural color materials from polydopamine black particles that mimic melanin granules. J. Mater. Chem. C, 2015, 3, 720–724. DOI: 10.1039/C4TC02383H. Kohri M., Yanagimoto K., Kawamura A., Fujii S., Matsuoka H., Kunitake T. Polydopamine-Based 3D Colloidal Photonic Materials: Structural Color Balls and Fibers from Melanin-Like Particles with Polydopamine Shell Layers. ACS Appl. Mater. Interfaces, 2018, 10, 7640–7648. DOI: 10.1021/acsami.7b03453. Kohri M., Yanagimoto K., Kawamura A., Fujii S., Matsuoka H., Kunitake T. Polydopamine-Based 3D Colloidal Photonic Materials: Structural Color Balls and Fibers from Melanin-Like Particles with Polydopamine Shell Layers. ACS Appl. Mater. Interfaces, 2018, 10, 7640–7648. DOI: 10.1021/acsami.7b03453. Kohri M. Progress in polydopamine-based melanin mimetic materials for structural color generation. Sci. Technol. Adv. Mater., 2020, 21, 833–848. DOI: 10.1080/14686996.2020.1852057. Kohri M. Progress in polydopamine-based melanin mimetic materials for structural color generation. Sci. Technol. Adv. Mater., 2020, 21, 833–848. DOI: 10.1080/14686996.2020.1852057. Zhu X., Yan B., Yan X., Zhang Y., Wang H. Fabrication of non-iridescent structural color on silk surface by rapid polymerization of dopamine. Prog. Org. Coat., 2020, 149, 105904. DOI: 10.1016/j.porgcoat.2020.105904. Zhu X., Yan B., Yan X., Zhang Y., Wang H. Fabrication of non-iridescent structural color on silk surface by rapid polymerization of dopamine. Prog. Org. Coat., 2020, 149, 105904. DOI: 10.1016/j.porgcoat.2020.105904. He L., Lai So V. L., Xin J. H. Dopamine polymerization-induced surface colouration of various materials. RSC Advances, 2014, 4, 20317–20322. DOI: https://doi.org/10.1039/C4RA00098F. He L., Lai So V. L., Xin J. H. Dopamine polymerization-induced surface colouration of various materials. RSC Advances, 2014, 4, 20317–20322. DOI: https://doi.org/10.1039/C4RA00098F. Jia W., Wang Q., Fan X., Wang X., Li R. Laccase-mediated in situ oxidation of dopa for bio-inspired coloration of silk fabric. RSC Advances, 2017, 7, 12977–12983. DOI: 10.1039/C6RA25533G. Jia W., Wang Q., Fan X., Wang X., Li R. Laccase-mediated in situ oxidation of dopa for bio-inspired coloration of silk fabric. RSC Advances, 2017, 7, 12977–12983. DOI: 10.1039/C6RA25533G. Nong Y., Zhou Z., Yuan J., Li X., Zhang Y., Liu Y., Wang X., Li R. Bio-Inspired Coloring and Functionalization of Silk Fabric via Laccase-Catalyzed Graft Polymerization of Arylamines. Fibers Polym., 2020, 21, 1927–1937. DOI: 10.1007/s12221-020-1044-9. Nong Y., Zhou Z., Yuan J., Li X., Zhang Y., Liu Y., Wang X., Li R. Bio-Inspired Coloring and Functionalization of Silk Fabric via Laccase-Catalyzed Graft Polymerization of Arylamines. Fibers Polym., 2020, 21, 1927–1937. DOI: 10.1007/s12221-020-1044-9. Citavi — From chaos to clarity. https://lumivero.com/products/citavi/. Accessed 30 Sep 2025. Citavi — From chaos to clarity. https://lumivero.com/products/citavi/. Accessed 30 Sep 2025. Tongyi Lab. Qwen3-Max (Version 3). Large language model. https://tongyi.aliyun.com/qwen/. Accessed 30 Sep 2025. Tongyi Lab. Qwen3-Max (Version 3). Large language model. https://tongyi.aliyun.com/qwen/. Accessed 30 Sep 2025. Kesornsit S., Jitjankarn P., Sajomsang W., Chairat M. Polydopamine‐coated silk yarn for improving the light fastness of natural dyes. Color. Technol., 2019, 135, 143–151. DOI: 10.1111/cote.12390. Kesornsit S., Jitjankarn P., Sajomsang W., Chairat M. Polydopamine‐coated silk yarn for improving the light fastness of natural dyes. Color. Technol., 2019, 135, 143–151. DOI: 10.1111/cote.12390. Ran J., He M., Li W., Zhang Y., Liu Y., Wang X., Li R. Growing ZnO Nanoparticles on Polydopamine-Templated Cotton Fabrics for Durable Antimicrobial Activity and UV Protection. Polymers, 2018, 10, 495. DOI: 10.3390/polym10050495. Ran J., He M., Li W., Zhang Y., Liu Y., Wang X., Li R. Growing ZnO Nanoparticles on Polydopamine-Templated Cotton Fabrics for Durable Antimicrobial Activity and UV Protection. Polymers, 2018, 10, 495. DOI: 10.3390/polym10050495. Pham T. L., Nguyen T. N., Bui V. C., Nguyen A. S., Dao T. H. Synthesis and study of Ag-TiO₂ nanoparticles for application in self-cleaning fabrics. ChemChemTech [Izv. Vyssh. Uchebn. Zaved. Khim. Khim. Tekhnol.], 2024, 67(1), 128–135. DOI: 10.6060/ivkkt.20246701.6962. Pham T. L., Nguyen T. N., Bui V. C., Nguyen A. S., Dao T. H. Synthesis and study of Ag-TiO₂ nanoparticles for application in self-cleaning fabrics. ChemChemTech [Izv. Vyssh. Uchebn. Zaved. Khim. Khim. Tekhnol.], 2024, 67(1), 128–135. DOI: 10.6060/ivkkt.20246701.6962. Ovchinnikov N. L., Vinogradov N. M., Gordina N. E., Kuznetsov D. V., Kuznetsova T. A., Kolesnikov A. V. Application of activating influences in obtaining TiO₂-pillared montmorillonite with improved photocatalytic properties. ChemChemTech [Izv. Vyssh. Uchebn. Zaved. Khim. Khim. Tekhnol.], 2024, 66(5), 59–71. DOI: 10.6060/ivkkt.20236605.6798. Ovchinnikov N. L., Vinogradov N. M., Gordina N. E., Kuznetsov D. V., Kuznetsova T. A., Kolesnikov A. V. Application of activating influences in obtaining TiO₂-pillared montmorillonite with improved photocatalytic properties. ChemChemTech [Izv. Vyssh. Uchebn. Zaved. Khim. Khim. Tekhnol.], 2024, 66(5), 59–71. DOI: 10.6060/ivkkt.20236605.6798. Zhu X., Wei T., Mia M. S., Li Y., Zhang Y., Wang H. Preparation of PS@PDA amorphous photonic structural colored fabric with vivid color and robust mechanical properties based on rapid polymerization of dopamine. Colloids Surf., A, 2021, 622, 126651. DOI: 10.1016/j.colsurfa.2021.126651. Zhu X., Wei T., Mia M. S., Li Y., Zhang Y., Wang H. Preparation of PS@PDA amorphous photonic structural colored fabric with vivid color and robust mechanical properties based on rapid polymerization of dopamine. Colloids Surf., A, 2021, 622, 126651. DOI: 10.1016/j.colsurfa.2021.126651. Tania I., Ali M., Azam M. S. In-situ Deposition of Ag Nanoparticles on Dopamine Pre-Modified Cotton Fabric and Analysis of Its Functional Mechanical and Dyeing Properties. J. Inorg. Organomet. Polym. Mater., 2021, 31, 1–12. DOI: 10.21203/rs.3.rs-324700/v1. Tania I., Ali M., Azam M. S. In-situ Deposition of Ag Nanoparticles on Dopamine Pre-Modified Cotton Fabric and Analysis of Its Functional Mechanical and Dyeing Properties. J. Inorg. Organomet. Polym. Mater., 2021, 31, 1–12. DOI: 10.21203/rs.3.rs-324700/v1. Wang Z., Wang Q., Dong X., Li D., Bai L., Wang X.-L., Wang Y.-Z., Song F. Photonic Cellulose Films with Vivid Structural Colors: Fabrication and Selectively Chemical Response. Biomacromolecules, 2022, 23, 1662 1671. DOI: https://doi.org/10.1021/acs.biomac.1c01567. Wang Z., Wang Q., Dong X., Li D., Bai L., Wang X.-L., Wang Y.-Z., Song F. Photonic Cellulose Films with Vivid Structural Colors: Fabrication and Selectively Chemical Response. Biomacromolecules, 2022, 23, 1662 1671. DOI: https://doi.org/10.1021/acs.biomac.1c01567.